ACME (https://en.wikipedia.org/wiki/Automated_Certificate_Manageme...) is still new, I don't believe any other certified CA implements it.
What is your use case? Maybe there's a better way.
Can I suggest that perhaps you could just start using alternative domains to avoid the rate limit?
Edit: also, how long since you requested the increase? They say it takes a few weeks.
ACME (https://en.wikipedia.org/wiki/Automated_Certificate_Manageme...) is still new, I don't believe any other certified CA implements it.
What is your use case? Maybe there's a better way.